Calculations of ZnO properties using the Heyd-Scuseria-Ernzerhof screened hybrid density functional

Author(s)
Jan Wrobel, Krzysztof J. Kurzydlowski, Kerstin Hummer, Georg Kresse, Jacek Piechota
Abstract

The Heyd-Scuseria-Ernzerhof (HSE) screened hybrid density functional has been proven to yield lattice constants and energy gaps of semiconductors in better agreement with experiment than standard local and semilocal exchange correlation functionals. The latter underestimate the band gaps of many semiconductors severely, i.e., in the case of ZnO the underestimation amounts to 75% of the experimental value. In this work, we report on the structure optimization and the study of the electronic band gap of ZnO in the wurtzite phase performed within density-functional theory using the semilocal Perdew-Burke-Ernzerhof as well as the HSE functional. Furthermore, the phonon-dispersion relations of ZnO and the dielectric and piezoelectric properties are calculated with both functionals and are compared to experimental findings.

Organisation(s)
Computational Materials Physics
External organisation(s)
Warsaw University of Technology, University of Warsaw
Journal
Physical Review B
Volume
80
No. of pages
8
ISSN
1098-0121
DOI
https://doi.org/10.1103/PhysRevB.80.155124
Publication date
2009
Peer reviewed
Yes
Austrian Fields of Science 2012
103009 Solid state physics, 103015 Condensed matter, 103025 Quantum mechanics, 103036 Theoretical physics
Portal url
https://ucrisportal.univie.ac.at/en/publications/fd33554a-4d9a-427f-a05e-17f42a3d3f85