BaPtSi3: A noncentrosymmetric BCS-like superconductor

Author(s)
Ernst Bauer, R T Khan, Herwig Michor, Esmaeil Royanian, Andrij Grytsiv, Nataliya Melnychenko-Koblyuk, Peter Franz Rogl, David Reith, Raimund Podloucky, Ernst Wilhelm Scheidt, Walter Wolf, Martijn Marsman
Abstract

By investigations of phase relations in the alloy system Ba-Pt-Si at 900 °C we observe the formation of the compound BaPtSi3, which crystallizes in the noncentrosymmetric BaNiSn3 structure type. Its space group is I4mm with the tetragonal lattice parameters a=0.44094(2)nm and c=1.0013(2)nm for the arc-melted compound annealed at 900 °C. The characterization of the physical properties of BaPtSi3 reveals a superconducting transition at 2.25 K with an upper critical field at T=0 K of [approximate]0.05 T. For analyzing the electronic structure, density-functional theory calculations are performed yielding very good agreement between theory and experiment for the structural properties. From relativistic electronic-structure calculations, Fermi surface nesting features are found for two characteristic double sets of bands. The spin-orbit splitting of the relativistic electronic bands is in general rather small at Fermi energy and, therefore, superconductivity adheres to an almost undisturbed BCS state.

Organisation(s)
Department of Physical Chemistry, Computational Materials Physics
External organisation(s)
Technische Universität Wien, Universität Augsburg, Materials Design s.a.r.l.
Journal
Physical Review B
Volume
80
ISSN
1098-0121
Publication date
2009
Peer reviewed
Yes
Austrian Fields of Science 2012
104017 Physical chemistry, 104011 Materials chemistry, 103018 Materials physics
Portal url
https://ucrisportal.univie.ac.at/en/publications/872682a4-44ea-4061-990d-c8b98bf1fd4a